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[triplenlace]

El mecanismo de Lindemann de las reacciones unimoleculares

La mayoría de las reacciones elementales en fase gaseosa son bimoleculares. Esto significa que la reacción se produce por el choque entre dos moléculas que se dirigen mutuamente una contra otra. Si la energía cinética que portan es suficiente, la colisión puede romper enlaces, con la eventual formación de otros. Pero existen también reacciones elementales unimoleculares, si bien, como vamos a…

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[rnomics]

Turn-on #RNA Mango Beacons for Trans-Acting Fluorogenic Nucleic Acid Detection [Article]

The Mango I and II RNA #aptamers have been widely used in vivo and in vitro as genetically-encodable fluorogenic markers that undergo large increases in fluorescence upon binding to their ligand, TO1-biotin. However, while studying nucleic acids sequences, it is often desirable to have trans-acting probes that induce fluorescence upon binding to a target sequence. Here, we rationally design three types of light-up RNA Mango Beacons based on a minimized Mango core, that induce fluorescence upon binding to a target RNA strand. Our first design is bi-molecular in nature and uses a DNA inhibition strand to prevent folding of the Mango #aptamer core until binding to a target RNA. Our second design is unimolecular in nature, and features hybridization arms flanking the core that inhibit G-quadruplex folding until refolding is triggered by binding to a target RNA strand. Our third design builds upon this structure, and incorporates a self-inhibiting domain into one of the flanking arms that deliberately binds to, and precludes folding of, the #aptamer core until a target is bound. This design separates G-quadruplex folding inhibition and RNA target hybridization into separate modules enabling a more universal unimolecular beacon design. All three Mango Beacons feature high contrasts and low costs, when compared to conventional molecular beacons, with excellent potential for in vitro and in vivo applications. http://rnajournal.cshlp.org/cgi/content/short/rna.079833.123v1?rss=1&utm_source=dlvr.it&utm_medium=tumblr

[testbankprovidersell]

Test Bank For Organic Chemistry Eighth Edition Peter Vollhardt

Table of Contents

1. Structure and Bonding in Organic Molecules 2. Structure and Reactivity: Acids and Bases, Polar and Nonpolar Molecules 3. Reactions of Alkanes: Bond-Dissociation Energies, Radical Halogenation, and Relative Reactivity 4. Cycloalkanes 5. Stereoisomers 6. Properties and Reactions of Haloalkanes: Bimolecular Nucleophilic Substitution 7. Further Reactions of Haloalkanes: Unimolecular Substitution and Pathways of Elimination 8. Hydroxy of Functional Group: Alcohols: Properties, Preparation, and Strategy of Synthesis 9. Further Reactions of Alcohols and the Chemistry of Ethers 10.Using Nuclear Magnetic Resonance Spectroscopy to Deduce Structure 11. Alkenes: Infrared Spectroscopy and Mass Spectrometry 12. Reactions to Alkenes 13. Alkynes: The Carbon 14. Delocalized Pi Systems: Investigation by Ultraviolet and Visible Spectroscopy   Interlude   15. Benzene and Aromaticity: Electrophilic Aromatic Substitution 16. Electrophilic Attack on Derivatives of Benzene: Substituents Control Regioselectivity 17. Aldehydes and Ketones: The Carbonyl Group 18. Enols, Enolates, and the Aldol Condensation: a,b-Unsaturated Aldehydes and Ketones 19. Carboxylic Acids 20. Carboxylic Acid Derivatives 21. Amines and Their Derivatives: Functional Groups Containing Nitrogen 22. Chemistry of the Benzene Substituents: Alkylbenzenes, Phenols, and Benzenamines 23. Ester Enolates and the Claisen Condensation: Synthesis of b-Dicarbonyl Compounds; Acyl Anion Equivalents 24. Carbohydrates: Polyfunctional Compounds in Nature 25. Heterocycles: Heteroatoms in Cyclic Organic Compounds 26. Amino Acids, Peptides, Proteins, and Nucleic Acids: Nitrogen-Containing Polymers in Nature Read the full article

[bscbooks]

#education #students #bscbooks #edtech #teaching #writers #chemistry

[cuetmocktest]

Haloalkanes & Haloarenes 08| Nucleophilic Unimolecular Substitution | Chemistry | CUET | Class 12 | CUET Mock

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[drachmann81woodward-blog]

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Science and Chemistry Classes

Changing the handedness of molecules

Researchers at Kanazawa University report in Proceedings of the National Academy of Sciences a responsive molecular system that, through chemical reactions, inverses its chirality before becoming racemic.

Molecules that have the ability to change their structure in response to a chemical or physical stimulus are called responsive molecules. This type of molecule plays an important role in signal transduction at the nanoscale. The typical time profile of a structural change of a responsive molecule follows an exponential relaxation. However, molecular systems with non-typical time responses, such as e.g. chemical oscillators (whose structure switches periodically between two states), offer advanced functionalities and are also intensively investigated. Shigehisa Akine and colleagues from Kanazawa University have now designed a particular responsive molecule in which the chirality ('handedness') changes in a non-exponential fashion. The achievement is a breakthrough in the field of responsive systems as the chirality change happens in a unimolecular system—not, as has often been the case before, in supramolecular assemblies.

The researchers' responsive molecule has six exchangeable sites; it can be written as [LCo3X6]3+, where X stands for a ligand at each of the six sites. The molecule has two forms, a 'left-handed' (abbreviated 'M') and a 'right-handed' (abbreviated 'P') version. In solution, the two forms will occur, in a given ratio. Akine and colleagues started from the molecule where X is a particular chiral amine labeled A (chiral means that the ligand and its mirror image cannot be superimposed, and amine refers to a type of molecular group containing nitrogen). In a methanol solution, the P/M ratio of [LCo3X6]3+ was 88:12, meaning that the right-handed version was dominant. The scientists then looked at what happened when exchanging the chiral A groups with piperidine (another, but achiral, amine).

Because of the achirality of the piperidine groups, the resulting [LCo3(piperidine)6]3+ solution should become 'racemic', which means that any effects of chirality are compensated. This is indeed what happened, but the researchers discovered that before reaching the racemic state after two days, the solution first switched from originally P-dominant to M-dominant after seven minutes, with maximum M-dominance after 60—120 minutes. Remarkably, a similar transient chirality inversion was not observed for the reverse reaction, [LCo3(piperidine)6]3+ to [LCo3X6]3+, for which the solution changed monotonically from racemic to P-dominant.

The transient chirality inversion in this study.  A right-handed helical cobalt(III) complex underwent the chirality inversion to give the left-handed form before complete racemization upon removal of the chiral source

Akine and colleagues note that their [LCo3X6]3+ responsive molecule is the first unimolecular platform displaying a transient chirality inversion, and that the unique chirality change happens on the timescale of minutes to hours, which could be potentially useful for time-dependent functional materials related to human activity. Quoting the scientists: "this result will provide an important insight into the science of autonomously driven materials."

[hassan-abouchadia]

The Collision Efficiency of Water in the Unimolecular Reaction CH4 (+ H2O) → CH3 + H (+ H2O): One-Dimensional and Two-Dimensional Solutions of the Low-Pressure-Limit Master Equation.

[madqueenalanna]

being a writer is needing to fact check a single thing and ending up combing through articles with names like “Mechanism of Thermal Unimolecular Decomposition of TNT (2,4,6-Trinitrotoluene):  A DFT Study”

#And yes I did struggle through the abstract of that study to get my answer #Writer's problems